Low‐dimensional material supported single‐atom catalysts for electrochemical CO <sub>2</sub> reduction

نویسندگان

چکیده

Converting CO2 emissions to valuable carbonaceous chemicals/fuels under mild conditions provides a sustainable way maintain carbon balance and alleviate the energy shortage. Low-dimensional material (LDM) supported single-atom catalysts (SACs) have been attracted significant attention for electrochemical reduction reaction (ECR) in recent years. This is mainly because integrating single-atoms LDMs can inherit advantages of themselves synergy effects between them are potential enhance ECR performance. In this review, we summarized strategies synthesizing LDM SACs ECR, different briefly introduced. Moreover, some optimization towards electroreduction highlighted. At end perspectives challenges provided.

برای دانلود باید عضویت طلایی داشته باشید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

CO oxidation on TiO2 supported gold catalysts

The aim within this project was to optimise the CO oxidation over TiO2 supported gold catalysts, focusing on two different preparation methods; deposition precipitation (DP) and photodeposition (PD), using different types of TiO2 and varying the theoretical gold loading. The catalyst were characterised with TEM (size) and ICP-AES (loading). For DP catalysts, the support is important for high ac...

متن کامل

Copper Catalysts Supported on CeMnO2 for CO Oxidation in Hydrogen-Rich Gas Streams

e"> The CeMnO2 supports were prepared via co-precipitation method by ammonia as <span style="font-size: 9p...

متن کامل

Electrochemical reduction of CO2 on graphene supported transition metals - towards single atom catalysts.

In this study, we have investigated the use of single metal atoms supported on defective graphene as catalysts for the electrochemical reduction of CO2 using the first-principles approach and the computational hydrogen electrode model. Reaction pathways to produce a variety of C1 products CO, HCOOH, HCHO, CH3OH and CH4 have been studied in detail for five representative transition metals Ag, Cu...

متن کامل

Graphyne-supported single Fe atom catalysts for CO oxidation.

Single atom catalysts (SACs) are highly desirable for the effort to maximize the efficiency of metal atom use. However, the synthesis of SACs is a major challenge that largely depends on finding an appropriate supporting substrate to achieve a well-defined and highly dispersed single atom. This work demonstrates that, based on the density functional theory (DFT) calculation, graphyne is a good ...

متن کامل

Metal Phosphate-Supported Pt Catalysts for CO Oxidation

Oxides (such as SiO₂, TiO₂, ZrO₂, Al₂O₃, Fe₂O₃, CeO₂) have often been used to prepare supported Pt catalysts for CO oxidation and other reactions, whereas metal phosphate-supported Pt catalysts for CO oxidation were rarely reported. Metal phosphates are a family of metal salts with high thermal stability and acid-base properties. Hydroxyapatite (Ca10(PO₄)₆(OH)₂, denoted as Ca-P-O here) also has...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

ژورنال

عنوان ژورنال: SmartMat

سال: 2022

ISSN: ['2766-8525', '2688-819X']

DOI: https://doi.org/10.1002/smm2.1101